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Dr Ines Graca,
Dr C Fernandez-Martin,
Dr Alan McCue
Applications accepted all year round
Self-Funded PhD Students Only
Aberdeen
United Kingdom
Analytical Chemistry
Chemical Engineering
Environmental Chemistry
Environmental Engineering
About the Project
These projects are open to students worldwide, but have no funding attached. Therefore, the successful applicant will be expected to fund tuition fees at the relevant level (home or international) and any applicable additional research costs. Please consider this before applying.
This experimental project will deal with the global challenge of mitigating CO2 emissions to the atmosphere, by using CO2 as a raw-material to produce fuels and fuel-precursors. It will involve the synthesis of materials, their characterisation and catalytic test under reaction conditions.
The hydrogenation of CO2 into oxygenates and/or hydrocarbons (methane, formic acid, methanol or dimethyl ether) has been the most investigated route to obtain fuels or fuel-precursors from this waste. However, this technology still faces some drawbacks: finding a sustainable hydrogen source and reduce the energy requirements for the chemical conversion of carbon dioxide.
The main goals of this project will be, thus, to develop heterogeneous catalysts with exceptional performance for the hydrogenation of CO2 using sustainable hydrogen sources, understand the behaviour of the catalysts and study the reaction mechanisms and kinetics involved. Catalysts will be optimised to achieve high conversion and selectivity for the desired products and to be active at relatively low temperature.
Beyond conventional thermal catalysis, the project can be expanded to include the development and use of innovative and future emerging energy technologies for the catalytic activation of molecules. These techniques will be used with the target of promoting heat and mass transfer and reducing energy input.
Essential Background:
Decisions will be based on academic merit. The successful applicant should have, or expect to obtain, a UK Honours Degree at 2.1 (or equivalent) in MEng/BEng in Chemical Engineering or any related discipline, such as BSc in Chemistry, Materials Science.
Desirable knowledge: Materials synthesis, materials characterisation, namely N2 physisorption, TGA, FTIR, XRD, gas chromatography, etc., reactor design and kinetics, heterogeneous catalysis. Microsoft Office package (especially Excel).
Application Procedure:
Formal applications can be completed online: https://www.abdn.ac.uk/pgap/login.php
You should apply for Engineering (PhD) to ensure your application is passed to the correct team for processing.
Please clearly note the name of the lead supervisor and project title on the application form. If you do not include these details, it may not be considered for the studentship.
Your application must include: A personal statement, an up-to-date copy of your academic CV, and clear copies of your educational certificates and transcripts.
Please note: you DO NOT need to provide a research proposal with this application.
If you require any additional assistance in submitting your application or have any queries about the application process, please don't hesitate to contact us at pgrs-admissions@abdn.ac.uk
Your application must include: A personal statement, an up-to-date copy of your academic CV, and clear copies of your educational certificates and transcripts.
Please note: you DO NOT need to provide a research proposal with this application.
If you require any additional assistance in submitting your application or have any queries about the application process, please don't hesitate to contact us at pgrs-admissions@abdn.ac.uk
Funding Notes
This is a self-funding project open to students worldwide. Our typical start dates for this programme are February or October.
Fees for this programme can be found here Finance and Funding | Study Here | The University of Aberdeen (abdn.ac.uk)
Additional research costs / bench fees of £3,000 per annum will also be required
References
[1] I. Graça, L.V. González, M.C. Bacariza, A. Fernandes, C. Henriques, J.M. Lopes, M.F. Ribeiro, CO2 hydrogenation into CH4 on NiHNaUSY zeolites Applied Catalysis B: Environmental, 147 (2014) 101-110.
[2] M.C. Bacariza, M. Biset-Peiró, I. Graça, J. Guilera, J. Morante, J.M. Lopes, T. Andreu, C. Henriques, DBD plasma-assisted CO2 methanation using zeolite-based catalysts: Structure composition-reactivity approach and effect of Ce as promoter, Journal of CO2 Utilization, 26 (2018) 202-211.
[3] M.C. Bacariza, I. Graça, J.M. Lopes, C. Henriques, Tuning Zeolite Properties towards CO2 Methanation: An Overview, ChemCatChem 11 (2019) 2388-2400.
[4] N. Westhuesand, J. Klankermayer, Transfer Hydrogenation of Carbon Dioxide to Methanol Using a Molecular Ruthenium-Phosphine Catalyst, ChemCatChem 11 (2019) 3371-3375.
[5] A. Stankiewicz, Energy Matters: Alternative Sources and Forms of Energy for Intensification of Chemical and Biochemical Processes, Chemical Engineering Research and Design 84 (2006) 511-521.
[2] M.C. Bacariza, M. Biset-Peiró, I. Graça, J. Guilera, J. Morante, J.M. Lopes, T. Andreu, C. Henriques, DBD plasma-assisted CO2 methanation using zeolite-based catalysts: Structure composition-reactivity approach and effect of Ce as promoter, Journal of CO2 Utilization, 26 (2018) 202-211.
[3] M.C. Bacariza, I. Graça, J.M. Lopes, C. Henriques, Tuning Zeolite Properties towards CO2 Methanation: An Overview, ChemCatChem 11 (2019) 2388-2400.
[4] N. Westhuesand, J. Klankermayer, Transfer Hydrogenation of Carbon Dioxide to Methanol Using a Molecular Ruthenium-Phosphine Catalyst, ChemCatChem 11 (2019) 3371-3375.
[5] A. Stankiewicz, Energy Matters: Alternative Sources and Forms of Energy for Intensification of Chemical and Biochemical Processes, Chemical Engineering Research and Design 84 (2006) 511-521.
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